塑料光催化降解回收处理技术的研究进展

赵慧莹, 李伟, 刘丰颉, 熊健, 吕学斌

PDF(1202 KB)
中国高校科技期刊信息汇聚平台
PDF(1202 KB)
塑料科技 ›› 2024, Vol. 52 ›› Issue (07) : 141-146. DOI: 10.15925/j.cnki.issn1005-3360.2024.07.030
综述

塑料光催化降解回收处理技术的研究进展

作者信息 +

Research Progress of Photocatalytic Degradation and Recycling of Plastics

Author information +
History +

摘要

为减轻塑料废弃物所带来的环境污染，对塑料光催化降解回收处理方式进行研究，从而利用太阳能光引发和光催化的降解机理将塑料转化为水和二氧化碳或进一步转化为氢气燃料和高值化学品。文章介绍催化剂特性、塑料和降解条件对光催化降解的影响，总结不同种类的无机金属、非金属材料以及有机-无机复合材料光催化剂在光催化降解回收处理中的应用，旨在通过催化剂的改性、与电催化、热催化、生物催化协同作用提升光催化效率。文章指出光催化降解塑料回收处理技术在预处理、处理后存在的问题，为废弃塑料的回收处理提供可靠依据和研究方向。

Abstract

In order to reduce the environmental pollution caused by plastic waste, research is being conducted on the photocatalytic degradation and recycling of plastics, utilizing the degradation mechanism of solar photoinitiation and photocatalysis to convert plastics into water and carbon dioxide, or further into hydrogen fuel and high-value chemicals. The article introduces the effects of catalyst characteristics, plastics, and degradation conditions on photocatalytic degradation, summarizes the applications of different types of inorganic metal, non-metal materials, and organic-inorganic composite photocatalysts in photocatalytic degradation and recycling, and aims to improve photocatalytic efficiency through catalyst modification and synergistic effects with electrocatalysis, thermocatalysis, and biocatalysis. The article points out the problems in the pre-treatment and post-treatment of photocatalytic degradation plastic recycling technology, providing a reliable basis and research direction for the recycling and treatment of waste plastics.

关键词

塑料降解 / 光催化降解 / 处理技术 / 协同处理

Key words

Plastic degradation / Photocatalytic degradation / Processing technology / Cooperative processing

中图分类号

X705

引用本文

EndNote

Ris (Procite)

Bibtex

导出引用
赵慧莹 , 李伟 , 刘丰颉 , 等. 塑料光催化降解回收处理技术的研究进展. 塑料科技. 2024, 52(07): 141-146 https://doi.org/10.15925/j.cnki.issn1005-3360.2024.07.030
ZHAO Hui-ying, LI Wei, LIU Feng-jie, et al. Research Progress of Photocatalytic Degradation and Recycling of Plastics[J]. Plastics Science and Technology. 2024, 52(07): 141-146 https://doi.org/10.15925/j.cnki.issn1005-3360.2024.07.030

参考文献

列表( 原文顺序 | 文献年度倒序 | 文中引用次数倒序 ) 可视化分析
1
XU Q, LI G, FANG L, et al. Enhanced formation of 6PPD-Q during the aging of tire wear particles in anaerobic flooded soils: The role of iron reduction and environmentally persistent free radicals[J]. Environmental Science & Technology, 2023, 57(14): 5978-5987.
本文引用 [1]
2
SUBRAMANIAN M. Plastics tsunami: Can a landmark treaty stop waste from choking the oceans?[J]. Nature, 2022, 611(7937): 650-653.
本文引用 [1]
3
BERGMANN M, COLLARD F, FABRES J, et al. Plastic pollution in the Arctic[J]. Nature Reviews Earth & Environment, 2022, 3(5): 323-337.
本文引用 [1]
4
LIU Z, SOKRATIAN A, DUDA A M, et al. Anionic nanoplastic contaminants promote Parkinson's disease-associated alpha-synuclein aggregation[J]. Research Square, 2023, DOI:10.1126/sciadv.adi8716.
本文引用 [1]
5
CHU S, ZHANG B W, ZHAO X, et al. Photocatalytic conversion of plastic waste: From photodegradation to photosynthesis[J]. Advanced Energy Materials, 2022, DOI: 10.1002/aenm.202200435.
本文引用 [1]
6
MOHARIR R V, KUMAR S. Challenges associated with plastic waste disposal and allied microbial routes for its effective degradation: A comprehensive review[J]. Journal of Cleaner Production, 2019, 208: 65-76.
本文引用 [1]
7
孙昱楠,张帆,李建园,等.废塑料处置与利用技术研究进展[J].中国工程科学,2023,25(3):182-196.
本文引用 [1]
8
苗开珍,孟娇龙,姜雪峰.塑料废弃物污染及降解的研究进展[J].华东师范大学学报:自然科学版,2023(1):170-176.
本文引用 [1]
9
孙静,熊礼龙,刘乐.聚乙烯塑料光降解研究进展[J].塑料科技,2022,50(7):120-123.
本文引用 [1]
10
KISCH H. Semiconductor photocatalysis: Princples and applications[M]. Angewandte Chemie, 2015, DOI: 10.1002/anie.201501876.
本文引用 [1]
11
JIANG D, YUAN H F, LIU Z, et al. Defect-anchored single-atom-layer Pt clusters on TiO2x/Ti for efficient hydrogen evolution via photothermal reforming plastics[J]. Applied Catalysis B: Environmental, 2023, DOI:10.1016/j.apcatb.2023.123081.
本文引用 [2]
12
GARCIA-MONTELONGO X L, MARTINEZ-DE LA CRUZ A, VAZQUEZ-RODRIGUEZ S, et al. Photo-oxidative degradation of TiO2/polypropylene films[J]. Materials Research Bulletin, 2014, 51: 56-62.
本文引用 [1]
13
XU J Z, YANG W, ZHANG C Q, et al. Photo-oxidation and biodegradation of polyethylene films containing polyethylene glycol modified TiO2 as pro-oxidant additives[J]. Polymer Composites, 2018, 39(S1): E531-E539.
本文引用 [1]
14
杨昌军,彭天右,邓克俭,等.固相光催化降解废弃塑料[J].化学进展,2011,23(5):874-879.
本文引用 [1]
15
TOFA T S, KUNJALI K L, PAUL S, et al. Visible light photocatalytic degradation of microplastic residues with zinc oxide nanorods[J]. Environmental Chemistry Letters, 2019, 17(3): 1341-1346.
本文引用 [1]
16
张妍,吴迪,李晨,等.半导体掺杂促进塑料可光降解性能的研究进展[J].应用化工,2020,49(5):1274-1277, 1283.
本文引用 [1]
17
LAM S M, SIN J C, ZENG H, et al. Green synthesis of Fe-ZnO nanoparticles with improved sunlight photocatalytic performance for polyethylene film deterioration and bacterial inactivation[J]. Materials Science in Semiconductor Processing, 2021, DOI:10.1016/j.mssp.2020.105574.
本文引用 [1]
18
LI H, LI J, AI Z H, et al. Oxygen vacancy-mediated photocatalysis of BiOCl: Reactivity, selectivity, and perspectives[J]. Angewandte Chemie-International Edition, 2018, 57(1): 122-138.
本文引用 [1]
19
PINO-RAMOS V H, BUCIO E, DIAZ D. Fast photocatalytic polypropylene degradation by nanostructured bismuth catalysts[J]. Polymer Degradation and Stability, 2021, DOI:10.1016/j.polymdegradstab.2021.109648.
本文引用 [1]
20
UEKERT T, KUEHNEL M F, WAKERLEY D W, et al. Plastic waste as a feedstock for solar-driven H2 generation[J]. Energy & Environmental Science, 2018, 11(10): 2853-2857.
本文引用 [1]
21
MENG X, PENG X, XUE J, et al. A biomass-derived, all-day-round solar evaporation platform for harvesting clean water from microplastic pollution[J]. Journal of Materials Chemistry A, 2021, 9(17): 11013-11024.
本文引用 [1]
22
CAO R, ZHANG M Q, HU C, et al. Catalytic oxidation of polystyrene to aromatic oxygenates over a graphitic carbon nitride catalyst[J]. Nature Communications, 2022, DOI:10.1038/s41467-022-32510-x.
本文引用 [1]
23
NINGSIH L A, LU P Y, ASHIMURA S, et al. Highly effective photocatalytic degradation of plastic film (LDPE) using ruthenium-incorporated g-C3N4 via the Norrish mechanism[J]. Chemical Engineering Journal, 2024, DOI:10.1016/j.cej.2023.148089.
本文引用 [1]
24
XING C W, YU G Y, ZHOU J, et al. Solar energy-driven upcycling of plastic waste on direct Z-scheme heterostructure of V-substituted phosphomolybdic acid/g-C3N4 nanosheets[J]. Applied Catalysis B-Environmental, 2022, DOI:10.1016/j.apcatb.2022.121496.
本文引用 [1]
25
WU Y F, WANG X J, KIRLIKOVALI K O, et al. Catalytic degradation of polyethylene terephthalate using a phase-transitional zirconium-based metal-organic framework[J]. Angewandte Chemie-International Edition, 2022, DOI:10.1002/anie.202117528.
本文引用 [1]
26
QIN J B, DOU Y B, WU F Y, et al. In-situ formation of Ag2O in metal-organic framework for light-driven upcycling of microplastics coupled with hydrogen production[J]. Applied Catalysis B—Environmental, 2022, DOI:10.1016/j.apcatb.2022.121940.
本文引用 [1]
27
蒋清梅,杨洋,文彬洁.溴氧化铋掺杂聚乙烯薄膜的可见光自降解性能研究[J].塑料科技,2021,49(6):66-69.
本文引用 [1]
28
LI W, ZHAO W, ZHU H, et al. State of the art in the photochemical degradation of (micro)plastics: From fundamental principles to catalysts and applications[J]. Journal of Materials Chemistry A, 2023, 11(6): 2503-2527.
本文引用 [1]
29
GOU N, YANG W Y, GAO S, et al. Incorporation of ultrathin porous metal-free graphite carbon nitride nanosheets in polyvinyl chloride for efficient photodegradation[J]. Journal of Hazardous Materials, 2023, DOI:10.1016/j.jhazmat.2023.130795.
本文引用 [1]
30
ZHOU D W, LUO H X, ZHANG F Z, et al. Efficient photocatalytic degradation of the persistent PET fiber-based microplastics over Pt nanoparticles decorated N-Doped TiO2 nanoflowers[J]. Advanced Fiber Materials, 2022, 4(5): 1094-1097.
本文引用 [1]
31
LLORENTE-GARCÍA B E, HERNANDEZ-LOPEZ J M, ZALDIVAR-CADENA A A, et al. First insights into photocatalytic degradation of HDPE and LDPE microplastics by a mesoporous N-TiO2 coating: Effect of size and shape of microplastics[J]. Coatings, 2020, DOI:10.3390/coatings10070658.
本文引用 [1]
32
MENG J, ZHOU Y, LI D, et al. Degradation of plastic wastes to commercial chemicals and monomers under visible light[J]. Science Bulletin, 2023, 68(14): 1522-1530.
本文引用 [1]
33
MAO R, LANG M, YU X, et al. Aging mechanism of microplastics with UV irradiation and its effects on the adsorption of heavy metals[J]. Journal of Hazardous Materials, 2020, DOI:10.1016/j.jhazmat.2020.122515.
本文引用 [1]
34
余小琴.光照对微塑料老化的影响过程和机制[D].杨凌:西北农林科技大学,2022.
本文引用 [1]
35
ARIZA-TARAZONA M C, VILLARREAL-CHIU J F, HERNÁNDEZ-LÓPEZ J M, et al. Microplastic pollution reduction by a carbon and nitrogen-doped TiO2: Effect of pH and temperature in the photocatalytic degradation process[J]. Journal of Hazardous Materials, 2020, DOI:10.1016/j.jhazmat.2020.122632.
本文引用 [1]
36
刘昕,戈钧,李春.光驱动微生物杂合系统提高生物制造水平[J].化工学报,2023,74(1):330-341.
本文引用 [1]
37
李亚峰,王志博,伍健伯.光电催化及其耦合技术的研究进展[J].现代化工,2023,43(10):30-35.
本文引用 [1]
38
KIM J, JANG J, HILBERATH T, et al. Photoelectrocatalytic biosynthesis fuelled by microplastics[J]. Nature Synthesis, 2022, 1(10): 776-786.
本文引用 [1]
39
MIAO Y X, ZHAO Y X, WATERHOUSE G I N, et al. Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions[J]. Nature Communications, 2023, DOI:10.1038/s41467-023-40005-6.
40
YE J, CHEN Y P, GAO C, et al. Sustainable conversion of microplastics to methane with ultrahigh selectivity by a biotic-abiotic hybrid photocatalytic system[J]. Angewandte Chemie-International Edition, 2022, DOI:10.1002/anie.202213244.
本文引用 [1]
41
LIU F, ZHUANG X J, DU Z F, et al. Enhanced photocatalytic performance by polarizing ferroelectric KNbO3 for degradation of plastic wastes under mild conditions[J]. Applied Catalysis B—Environmental, 2022, DOI:10.1016/j.apcatb.2022.121897.
本文引用 [1]
42
LIU Y, ZHANG C, FENG J, et al. Integrated photochromic-photothermal processes for catalytic plastic upcycling[J]. Angewandte Chemie—International Edition, 2023, DOI: 10.1002/anie.202308930.
本文引用 [1]
43
LOU X, GAO X, LIU Y, et al. Highly efficient photothermal catalytic upcycling of polyethylene terephthalate via boosted localized heating[J]. Chinese Journal of Catalysis, 2023, 49: 113-122.
本文引用 [1]
44
THEW X E C, LO S C, RAMANAN R N, et al. Enhancing plastic biodegradation process: Strategies and opportunities[J]. Critical Reviews in Biotechnology, 2023, DOI: 10.1080/07388551.2023.2170861.
本文引用 [1]
45
YUAN Y B, ZHOU W K, LIANG Q F, et al. Advances in biodegradation of polyolefin plastics[J]. Sheng Wu Gong Cheng Xue Bao, 2023, 39(5): 1930-1948.
本文引用 [1]
46
李凤红,李鹏珍,笪伟,等.光-生物可降解LDPE/纳米TiO2/TPS复合膜材料的制备及性能研究[J].化工新型材料,2023,51(1):290-295.
本文引用 [1]
47
钟宛真,单斌,谭伟强,等.水中微塑料光催化处理的进展[J].精细化工,2023,40(6):1176-1186.
本文引用 [1]
48
LI W Y, WU C J, XIONG Z, et al. Self-driven magnetorobots for recyclable and scalable micro/nanoplastic removal from nonmarine waters[J]. Science Advances, 2022, DOI:10.1126/sciadv.ade1731.
本文引用 [1]
49
BELADI-MOUSAVI S M, HERMANOVA S, YING Y, et al. A maze in plastic wastes: Autonomous motile photocatalytic microrobots against microplastics[J]. ACS Applied Materials & Interfaces, 2021, 13(21): 25102-25110.
本文引用 [1]
50
KIM J, MAYORGA-MARTINEZ C C, PUMERA M. Magnetically boosted 1D photoactive microswarm for COVID-19 face mask disruption[J]. Nature Communications, 2023, DOI:10.1038/s41467-023-36650-6.
本文引用 [1]

基金

西藏自治区科技计划项目(XZ202101ZY0012G)
西藏自治区科技计划项目(XZ202202YD0027C)
西藏自治区科技计划项目(XZ202301ZY0020G)
西藏大学2023年国家级大学生创新训练项目(202310694014)
中央支持地方高校专项资金(藏财预指（2023）01)
中央支持地方高校专项资金(藏财预指（2024）01）)
西藏大学人才发展激励计划——青年学者项目

评论

PDF(1202 KB)

Accesses

Citation

Detail
段落导航
相关文章
Copyright 中国高校科技期刊信息汇聚平台 2024-2025
技术支持：北京玛格泰克科技发展有限公司
京ICP备05021913号-19

/

〈 〉